E. V. D. van Loef, P. Dorenbos, C. W. E. van Eijk, K. W. Krämer and H. U. Güdel
Properties and mechanism of scintillation in LuCl3:Ce3+ and LuBr3:Ce3+ crystals
Nucl. Instr. and Methods Phys. Res. A 496, 138-145 (2003)
Abstract:
The optical and scintillation properties of pure LuCl3,
LuCl3:0.45%, 2%, 4%, 10% Ce3+, LuBr3:0.021%,
0.46%, 0.76%, 2.5%, and 8% Ce3+ are studied under X-ray and g-ray
excitation. The highest light yield of 29,000±3000 photons per MeV (ph/MeV) of
absorbed g-ray
energy was measured for LuBr3:0.021% Ce3+. Energy
resolutions obtained with a Hamamatsu R1791 photomultiplier tube (PMT) range
from 6.0±0.5% to 18±2% for LuBr3:8% Ce3+ and
LuCl3:0.45% Ce3+, respectively. For both
LuCl3:Ce3+ and LuBr3:Ce3+, binary
electron–hole diffusion was proposed as the dominant scintillation mechanism. At
lower irradiation temperatures, VK diffusion is probably more
important in the case of LuBr3:Ce3+.